Brownian diffusion of fibers

Tian, L, Ahmadi, G and Tu, J 2016, 'Brownian diffusion of fibers', Aerosol Science and Technology, vol. 50, no. 5, pp. 474-486.

Document type: Journal Article
Collection: Journal Articles

Title Brownian diffusion of fibers
Author(s) Tian, L
Ahmadi, G
Tu, J
Year 2016
Journal name Aerosol Science and Technology
Volume number 50
Issue number 5
Start page 474
End page 486
Total pages 13
Publisher Taylor and Francis
Abstract Motion of nanoparticles suspended in fluids are dominated by Brownian diffusiona physical property well understood following the work by Einstein in 1905. While theoretical derivation and experimental measurement of the diffusion coefficients for spherical particles are well developed, such information is lacking for non-spherical particles as the coupled rotational and translational motion hinders a clear description of the overall diffusive outcome. In this study, the Brownian diffusion of elongated nano-fibers is investigated numerically. Motion of the nano-fiber is resolved by solving the system of equations governing its coupled translational and rotational motion. To isolate the Brownian diffusion from other diffusive forces, test fibers are immersed in an unbounded quiescent fluid where only the hydrodynamic drag and Brownian forces are present. The study allows a close look at the Brownian diffusion of nano-fibers with respect to the translation, rotation, coupling, and how the rotation affects the particle's macroscopic diffusion properties. In this study, the Brownian diffusion of ellipsoidal particles are studied. The translational and the rotational Brownian motions and their coupling are included in the analysis. Particular attention was given to the rotational relaxation time in determining the non-spherical particle's isotropic and anisotropic diffusive properties. Theoretical and semi-empirical equations are developed to quantify the diffusion coefficients of nano-fibers. The predications are compared with available experimental data. The comparison to the analytic solution in the limiting case of a sphere is with excellent accuracy. The study opens up new approaches for studying fundamental diffusive processes of non-spherical elongated particles that are abundant in natural environment.
Subject Computational Fluid Dynamics
DOI - identifier 10.1080/02786826.2016.1165340
Copyright notice © 2016 American Association for Aerosol Research
ISSN 0278-6826
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Citation counts: TR Web of Science Citation Count  Cited 5 times in Thomson Reuters Web of Science Article | Citations
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